You searched for: “most unalloyed”
unalloyed (adjective), more unalloyed, most unalloyed
Pertaining to something that is not mixed with anything else: Mary had unalloyed pleasure when her daughter gave birth to her first baby.

There are some unalloyed metals that are not blended nor mingled with others; for example, copper.

Complete and pure joy or happiness.
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This entry is located in the following unit: English Words in Action, Group U (page 1)